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61.
Food chain enrichment of organochlorine compounds and mercury in clean and polluted lakes of Finland
Jaakko Passivirta Jukka Särkkä Kari Surma-Aho Tarmo Humppi Tauno Kuokkanen Markku Marttinen 《Chemosphere》1983,12(2):239-252
Lakes polluted by pulp mill and urban wastes including chlorobleaching of pulp, semipolluted lakes and reference lakes in nearly natural condition in Central Finland were studied for contents of mercury, methyl mercury and organochlorine compounds in sediment, plankton, roach and pike. Chlorobleaching had caused a 30-fold concentration of Hg in bottom sediment related to that of the purest reference lake. This was not reflected to the mercury levels in fish which were highest at one natural condition (humic) lake and rather high also at semipolluted lake Päijänne. Mercury in fish was shown to be mostly methylated but not completely and its time trends could be estimated. Chloroform showed no but carbon tetrachloride, tetrachloroethylene and chlorinated cymenes significant bioaccumulation in fish. Levels of chlorophenols from bleaching had strongly decreased but pentachlorophenol and 2,3,4,6-tetrachlorphenol levels remained related to earlier results. Using fat basis attenuated the power of estimation of food chain enrichment by a three throphic level model for lipohilic biocides and a strong proof was obtained of the enrichment of hexachlorobenzene. The time trends at Päijänne were decreasing for mercury and DDE but increasing for PCB. 相似文献
62.
Rask M Saxén R Ruuhijärvi J Arvola L Järvinen M Koskelainen U Outola I Vuorinen PJ 《Journal of environmental radioactivity》2012,103(1):41-47
We summarize the patterns of 137Cs activity concentrations and transfer into fish and other biota in four small forest lakes in southern Finland during a twenty-year period following the Chernobyl accident in April 1986. The results from summer 1986 showed fastest accumulation of 137Cs into planktivorous fishes, i.e. along the shortest food chains. Since 1987, the highest annual mean values of 137Cs have been recorded in fish occupying the highest trophic levels, for perch (Perca fluviatilis) 13,600 Bq/kg (ww) and for pike (Esox lucius) 20,700 Bq/kg (ww). At the same time, activity concentrations of 137Cs in crustacean zooplankton and Asellus aquaticus have ranged between 1000 and 19,500 Bq/kg (dw). In 2006, 5-28% of the 1987 137Cs activity concentration levels were still present in perch and pike. Since 1989 their 137Cs activity concentrations in oligohumic seepage lakes have remained significantly higher than in polyhumic drainage lakes due to the increased transfer of 137Cs into fish in the seepage lakes with lower electrolyte concentrations, longer water retention times and lower sedimentation rate. 相似文献